MORTALIDAD POR TUMORES DE PULMÓN, LARINGE Y …



Title of the manuscript: "Cancer mortality in towns in the vicinity of installations for the production of cement, lime, plaster, and magnesium oxide."Supplementary DataThis document is available as supplementary data for inclusion as online documentation. It includes:Table S1, showing the list of tumors analyzed and their codes as per the International Classification of Diseases-9th Revision (ICD-9) and 10th Revision (ICD-10).Table S2, showing observed and expected cases, and the relative risk of dying from cancer in towns situated at a distance of 5 km or less from installations for the production of cement, lime, plaster, and magnesium oxide as a whole, estimated using BYM models.Table S3, showing Moran’s I statistics and p-values for spatial autocorrelation analyses, by tumor type.Table S4, showing observed and expected cases, and the relative risk of dying from cancer in towns situated at a distance of 5 km or less from installations for the production of cement, lime, plaster, and magnesium oxide as a whole, estimated using BYM models and shown with a breakdown by category of manufactured product.Table S5, showing a description of industrial facilities analyzed in the paper, including the following information: PRTR code; category of industrial activity; province and municipality where the respective facilities are located; and pollutants released in the last twelve years to both air and water. Table S6, showing the types of substances and amounts released to air by Spanish installations for the production of cement, lime, plaster, and magnesium oxide (IPPC, 2009).Table S7, showing the types of substances and amounts released to water by Spanish installations for the production of cement, lime, plaster, and magnesium oxide (IPPC, 2009).Figure S1, showing geographic distribution of Spanish installations for the production of cement, lime, plaster, and magnesium oxide.Supplementary data, Table S1.TumorICD-9ICD-10Malignant neoplasm of lip, oral cavity, and pharynx 140-149C00-C14Malignant neoplasm of esophagus150C15Malignant neoplasm of stomach151C16Malignant neoplasm of small intestine, including duodenum152C17Malignant neoplasm of colon, rectum, rectosigmoid junction, and anus153-154, 159.0C18-C21Malignant neoplasm of liver, primary155.0C22.0Malignant neoplasm of gallbladder and extrahepatic bile ducts156C23-C24Malignant neoplasm of pancreas157C25Malignant neoplasm of retroperitoneum and peritoneum158C45.1, C48Malignant neoplasm of nasal cavities, middle ear, and accessory160C30-C31Malignant neoplasm of larynx161C32Malignant neoplasm of trachea, bronchus, and lung162C33-C34Malignant neoplasm of pleura163C38.4, C45.0Malignant neoplasm of bone and articular cartilage170C40-C41Malignant neoplasm of connective and other soft tissue171C49Malignant melanoma of skin172C43Other malignant neoplasm of skin173C44Malignant neoplasm of female breast174C50Malignant neoplasm of other and unspecified female genital organs (vulva and vagina)184C51, C52Malignant neoplasm of uterus179-182C53-C55Malignant neoplasm of ovary and other uterine adnexa183C56, C57Malignant neoplasm of prostate185C61Malignant neoplasm of testis186C62Malignant neoplasm of bladder188C67Malignant neoplasm of kidney and other and unspecified urinary organs189C64-C66, C68Malignant neoplasm of brain191C71Malignant neoplasm of other and unspecified parts of nervous system192C70, C72Malignant neoplasm of thyroid gland193C73Malignant neoplasm of other and ill-defined sites, or without specification of site195-199C76-C80Non-Hodgkin lymphoma200, 202C82-C85, C96Hodgkin lymphoma201C81Multiple myeloma and immunoproliferative neoplasms203C90Leukemia204-208C91-C95Supplementary data, Table S2.?TaObsbExpcRRd95%CrIe??TaObsbExpcRRd95%CrIeAll cancersf?????Melanoma????Total1484312641470.01.031.00-1.06Total148387355.01.080.95-1.22Men1482717925845.51.041.01-1.07Men148205190.31.060.89-1.25Women1481594715624.41.031.00-1.06Women148182164.81.110.92-1.32??Oral and pharyngeal cancerSkin cancer?Total14812391067.71.040.94-1.14Total148191205.21.090.90-1.31Men1481044885.01.040.93-1.15Men148103109.41.100.85-1.38Women148195182.71.020.85-1.21Women1488895.81.060.80-1.37??Oesophageal cancerBreast cancer?Total148993847.91.040.94-1.15Women14828302787.71.020.96-1.09Men148873736.21.070.96-1.19?Women148120111.70.890.69-1.13Vulvar and vaginal cancer??Women148159153.51.070.88-1.29Stomach cancer?Total14825492747.01.070.99-1.16Uterine cancer?Men14815991684.01.091.00-1.18Women148900861.31.030.93-1.13Women1489501063.01.040.94-1.15??Ovarian cancer?Small intestine cancerWomen148799865.20.970.88-1.06Total1486163.20.930.66-1.26?Men1483634.41.010.67-1.44Prostate cancer?Women1482528.80.870.53-1.32Men14822792396.10.980.92-1.04??Colorectal cancerTesticular cancer?Total14857785524.61.081.03-1.13Men1481621.60.850.45-1.40Men14832143081.71.071.01-1.14?Women14825642443.01.101.03-1.16Bladder cancer??Total14820301846.61.071.00-1.16Liver cancerMen14817051521.01.111.03-1.20Total14811841125.71.050.94-1.17Women148325325.50.960.83-1.10Men148865818.71.060.93-1.19?Women148319307.01.030.85-1.23Renal cancer??Total148870804.41.040.94-1.14Gallbladder cancerMen148574533.11.030.92-1.15Total148662612.81.090.98-1.22Women148296271.41.090.94-1.26Men148238209.71.211.02-1.42?Women148424403.21.040.91-1.19Brain cancer??Total14811581103.81.060.97-1.15Pancreatic cancerMen148650614.41.060.96-1.15Total14818581951.40.960.89-1.03Women148508489.41.050.93-1.17Men1489901041.10.940.86-1.03?Women148868910.30.960.87-1.05Cancer of other parts of nervous system?Total14830782796.91.071.00-1.14Peritoneal cancerMen14818021562.01.131.04-1.21Total148126110.61.220.96-1.53Women14812761234.91.010.93-1.09Men1486650.21.621.15-2.20?Women1486060.50.940.69-1.26Thyroid cancer??Total148131125.81.030.82-1.26Nasal cancerMen1484542.41.030.72-1.41Total1484043.11.030.69-1.46Women1488683.41.020.78-1.31Men1482430.20.870.52-1.33?Women1481612.91.350.70-2.29Ill-defined tumors??Total14830782796.91.071.00-1.14Laryngeal cancerMen14818021562.01.131.04-1.21Total148831821.51.020.91-1.13Women14812761234.91.010.93-1.09Men148797791.41.020.91-1.13?Women1483430.01.100.71-1.60Non-Hodgkin’s lymphoma??Total14811501093.30.980.89-1.07Lung cancerMen148612572.21.010.90-1.13Total14889648490.51.030.98-1.08Women148538521.00.930.82-1.05Men14879007484.51.040.98-1.10?Women14810641006.10.970.88-1.07Hodgkin’s lymphoma??Total148120115.41.020.81-1.25Pleural cancerMen1486065.30.900.66-1.18Total148158100.81.501.15-1.91Women1486050.11.190.86-1.58Men14811071.71.711.24-2.28?Women1484829.11.220.80-1.77Myeloma??Total148769694.41.060.97-1.17Bones cancerMen148378341.41.100.97-1.25Total148129142.70.870.71-1.06Women148391353.01.050.92-1.19Men1486583.30.700.52-0.91?Women1486459.41.170.86-1.55Leukemia??Total15514601363.61.060.99-1.14Connective and soft tissue cancerMen155815757.51.070.98-1.17Total148193202.90.970.81-1.15Women155645606.11.060.95-1.17Men148101103.91.000.79-1.24?Women1489299.00.970.74-1.23??????? aNumber of towns situated at ≤5 km from installations for the production of cement, lime, plaster, and magnesium oxide as a whole.bObserved deaths.cExpected deaths.dRRs adjusted for population size, percentages of illiteracy, farmers and unemployed persons, average persons per household, and mean incomee95% credible interval.fSum of the 33 types of cancer analyzed.Supplementary data, Table S3.TumorSexObservedMoran's I statisticP-valueAll cancersaTotal8930600.136092600.0001All cancersaMen5612250.133909400.0001All cancersaWomen3318350.038672700.0006Oral cavity-pharynxTotal219780.028515270.0039Oral cavity-pharynxMen181360.032814450.0031Oral cavity-pharynxWomen3842-0.004976930.4660EsophagusTotal177600.014974620.0725EsophagusMen153770.013460980.0979EsophagusWomen23830.002178310.7441StomachTotal596710.059193670.0001StomachMen367540.024062380.0073StomachWomen229170.029363690.0049Small intestineTotal13640.023217880.0163Small intestineMen7440.003242120.5262Small intestineWomen6200.003571490.3594Colon-rectumTotal1208410.033487000.0004Colon-rectumMen680950.021789900.0131Colon-rectumWomen527460.003765310.6319LiverTotal242550.032729910.0012LiverMen176090.036501950.0014LiverWomen66460.001749380.8100GallbladderTotal134670.008997940.2574GallbladderMen46820.004503730.5436GallbladderWomen8785-0.003200820.6723PancreasTotal419180.006626720.4224PancreasMen22328-0.001786630.8569PancreasWomen195900.004160460.5961PeritoneumTotal2347-0.007436440.2266PeritoneumMen1066-0.001811220.7607PeritoneumWomen1281-0.006041240.2213NasalTotal908-0.003546550.4886NasalMen636-0.002366830.6296NasalWomen272-0.002826670.2493LarynxTotal172970.008719220.2829LarynxMen166740.008308980.3049LarynxWomen623-0.004605730.1950LungTotal1810270.138619700.0001LungMen1601040.149220800.0001LungWomen20923-0.000761820.9473PleuraTotal21560.009914730.1093PleuraMen15380.011313360.0688PleuraWomen618-0.001200120.8281BoneTotal29210.006202730.3433BoneMen17020.010738170.0778BoneWomen1219-0.004035570.4080Connective and soft tissueTotal4182-0.004227380.5665Connective and soft tissueMen2148-0.002423060.7297Connective and soft tissueWomen2034-0.001702390.7879MelanomaTotal7401-0.003599930.6458MelanomaMen3987-0.003147650.6672MelanomaWomen34140.002522780.7087SkinTotal46320.006032350.3792SkinMen24980.004569810.4815SkinWomen21340.007011610.2312BreastWomen578300.018167820.0409Vulva and vaginaWomen3355-0.007282990.2742UterusWomen180800.010813230.1745OvaryWomen180460.001803270.8134Prostate glandMen557720.023954050.0060TestisMen425-0.000834720.8640BladderTotal412820.020998620.0140BladderMen341070.023005390.0092BladderWomen7175-0.002492270.7499KidneyTotal173410.003653530.6497KidneyMen115320.005488410.4631KidneyWomen5809-0.000155710.9937BrainTotal226890.000635340.9354BrainMen12622-0.011037040.1687BrainWomen100670.008706120.2573Other central nervous systemTotal801-0.005650160.1698Other central nervous systemMen400-0.003317810.2930Other central nervous systemWomen401-0.001244130.7755Thyroid glandTotal27110.004137720.5100Thyroid glandMen911-0.001973590.7459Thyroid glandWomen18000.003858050.4953Ill-definedTotal606380.017332770.0393Ill-definedMen339680.009268130.2712Ill-definedWomen266700.009119070.2623Non-Hodgkin’s lymphomaTotal233380.007246690.3802Non-Hodgkin’s lymphomaMen122290.002547730.7342Non-Hodgkin’s lymphomaWomen111090.012694860.1000Hodgkin’s lymphomaTotal2379-0.003862220.5652Hodgkin’s lymphomaMen1345-0.005829300.2573Hodgkin’s lymphomaWomen1034-0.002236280.6798MyelomaTotal151780.012929080.1116MyelomaMen7541-0.001044810.8915MyelomaWomen76370.008925360.2204LeukemiaTotal290700.003799370.6310LeukemiaMen162950.011994550.1279LeukemiaWomen12775-0.008888750.2602aSum of the 33 types of cancer analyzed.Supplementary data, Table S4.??Total?Men?WomenType of manufactured productTaObsbExpcRRd95%CrIe?ObsbExpcRRd95%CrIe?ObsbExpcRRd95%CrIeAll cancersf?Cement873666735128.61.041.01-1.072314021834.11.051.01-1.091352713294.51.020.99-1.05Lime4848954784.91.030.98-1.0930853027.31.020.96-1.0918101757.61.050.98-1.11Plaster11883871.70.990.88-1.11533557.60.960.83-1.10350314.11.120.98-1.28Magnesium oxide12944.20.730.47-1.051830.20.700.40-1.101114.00.830.41-1.40Multiple pollutant categories1652640.60.990.81-1.20403396.31.030.82-1.29249244.30.970.80-1.17??Oral and pharyngeal cancer?Cement871064907.91.010.90-1.12903752.41.020.91-1.14161155.50.970.80-1.17Lime48135119.41.150.93-1.4110699.01.080.85-1.342920.51.450.95-2.06Plaster112223.61.150.68-1.771919.91.200.68-1.8933.80.790.17-1.92Magnesium oxide111.01.150.04-4.3410.91.430.05-5.3900.200-infMultiple pollutant categories11715.71.170.60-2.001512.81.250.61-2.1922.90.700.10-1.96??Oesophageal cancer?Cement87876720.61.070.96-1.20773625.51.110.98-1.2410395.10.880.67-1.13Lime488895.70.880.68-1.117583.10.880.67-1.121312.60.930.48-1.57Plaster112018.31.370.79-2.121716.01.320.74-2.1232.21.580.33-3.93Magnesium oxide120.82.510.33-7.1720.72.810.37-8.0400.100-infMultiple pollutant categories1712.60.580.22-1.16610.80.590.20-1.2211.80.550.02-2.07??Stomach cancer?Cement8721482324.91.080.99-1.1813541422.01.100.99-1.21794902.91.050.94-1.17Lime48313319.11.070.91-1.25197198.01.130.94-1.35116121.10.990.78-1.23Plaster115257.11.010.70-1.403136.10.940.60-1.372121.01.070.63-1.64Magnesium oxide133.01.040.22-2.6012.00.490.02-1.8521.02.160.28-6.18Multiple pollutant categories13342.90.900.51-1.461625.90.710.35-1.241717.01.210.62-2.09??Small intestine cancer?Cement875353.50.930.64-1.283429.01.120.73-1.601924.50.770.44-1.22Lime4867.30.890.32-1.7824.00.540.07-1.5243.31.270.34-2.86Plaster1111.30.860.04-3.1800.700-inf10.61.820.06-6.87Magnesium oxide100.100-inf00.000-inf00.000-infMultiple pollutant categories111.01.200.05-4.6400.500-inf10.52.270.08-8.68??Colorectal cancer?Cement8749184673.91.091.03-1.1527132598.11.071.00-1.1422052075.71.111.04-1.19Lime48643644.11.050.95-1.16379366.11.080.95-1.26264278.01.010.87-1.15Plaster11121113.41.140.90-1.406265.51.080.80-1.425947.81.270.94-1.65Magnesium oxide146.10.760.21-1.7133.80.900.19-2.2112.30.520.02-1.97Multiple pollutant categories19287.20.970.70-1.295748.11.090.75-1.523539.10.850.56-1.21??Liver cancer?Cement871014954.41.040.92-1.18735693.21.030.90-1.18279261.21.050.86-1.28Lime48128129.61.080.84-1.369794.81.150.88-1.473134.80.980.61-1.45Plaster112423.41.070.62-1.701817.61.140.62-1.8765.91.000.34-2.10Magnesium oxide111.21.530.06-5.7910.91.900.07-7.2100.300-infMultiple pollutant categories11717.11.020.46-1.911412.31.140.51-2.1734.80.580.11-1.56??Gallbladder cancer?Cement87568519.11.120.99-1.26208176.61.271.06-1.51360342.61.050.90-1.21Lime487071.20.970.73-1.242325.10.980.61-1.444746.10.990.71-1.33Plaster111312.11.150.60-1.9124.40.530.07-1.50117.71.420.69-2.46Magnesium oxide110.71.390.05-5.1300.300-inf10.42.230.08-8.42Multiple pollutant categories1109.81.090.49-2.0053.31.610.50-3.4756.50.850.26-1.86??Pancreatic cancer?Cement8715951655.80.970.89-1.04856881.30.960.87-1.06739774.50.950.85-1.05Lime48203223.30.950.81-1.11103120.40.880.70-1.08100102.91.030.82-1.27Plaster113640.30.970.66-1.341722.50.800.46-1.251917.71.180.69-1.80Magnesium oxide132.01.380.29-3.3821.11.690.22-4.8010.81.060.04-4.00Multiple pollutant categories12130.10.690.40-1.081215.70.740.36-1.26914.40.630.28-1.15??Peritoneal cancer?Cement8710494.01.160.90-1.485642.51.611.12-2.244851.50.880.62-1.21Lime481712.51.550.87-2.4675.81.610.62-3.20106.81.390.65-2.45Plaster1122.30.940.12-2.6901.100-inf21.21.590.20-4.51Magnesium oxide110.19.760.37-37.3110.120.150.79-78.6800.100-infMultiple pollutant categories121.71.250.16-3.6920.83.630.45-11.2100.900-inf??Nasal cancer?Cement873636.61.090.72-1.572125.60.890.52-1.401511.01.500.77-2.57Lime4834.90.730.16-1.8023.50.680.09-1.9411.40.780.03-2.93Plaster1100.900-inf00.700-inf00.300-infMagnesium oxide100.000-inf00.000-inf00.000-infMultiple pollutant categories110.72.000.10-7.2710.52.930.11-11.3100.200-inf??Laryngeal cancer?Cement87718697.31.030.92-1.16687671.71.030.91-1.163125.61.170.74-1.73Lime489493.41.010.79-1.279190.11.010.78-1.2733.30.960.20-2.37Plaster111417.70.960.50-1.591417.10.980.51-1.6300.600-infMagnesium oxide110.91.410.05-5.3010.81.450.05-5.4900.000-infMultiple pollutant categories1412.20.390.10-0.90411.70.410.11-0.9500.500-inf??Lung cancer?Cement8776727197.91.040.98-1.1067506340.51.050.99-1.12922857.40.970.87-1.08Lime48977974.31.020.92-1.13864862.71.010.90-1.12113111.71.070.84-1.32Plaster11173181.80.930.73-1.15157160.90.950.73-1.201620.90.800.44-1.29Magnesium oxide129.00.300.04-0.8528.10.350.05-1.0000.800-infMultiple pollutant categories1140127.61.130.79-1.57127112.21.210.82-1.731315.30.740.36-1.31??Pleural cancer?Cement8714385.61.591.19-2.0610060.71.861.33-2.524324.81.220.78-1.81Lime48811.50.850.35-1.6168.30.940.33-1.9423.30.660.09-1.91Plaster1162.13.441.14-7.4041.53.120.77-7.6320.65.100.64-14.99Magnesium oxide100.100-inf00.100-inf00.000-infMultiple pollutant categories111.50.610.02-2.3901.100-inf10.41.920.07-7.53??Bones cancer?Cement87109120.70.870.69-1.085470.30.690.50-0.915550.31.200.86-1.61Lime481016.30.610.29-1.0559.60.490.16-1.0256.70.790.25-1.65Plaster1163.51.660.61-3.2822.10.850.11-2.3941.43.160.85-7.14Magnesium oxide100.100-inf00.100-inf00.000-infMultiple pollutant categories142.21.820.49-4.1241.23.030.81-6.9600.900-inf??Connective and soft tissue cancer?Cement87165172.10.980.80-1.178687.81.000.77-1.267984.30.980.73-1.26Lime481922.90.830.49-1.271111.90.980.48-1.65811.00.730.31-1.34Plaster1174.71.670.66-3.1922.50.840.11-2.3752.22.680.86-5.66Magnesium oxide100.200-inf00.100-inf00.100-infMultiple pollutant categories123.00.700.09-1.9921.61.350.17-3.8301.500-inf??Melanoma?Cement87323300.91.050.91-1.20168160.81.020.84-1.22155140.11.110.90-1.34Lime483840.30.960.67-1.312121.90.990.61-1.481718.40.940.54-1.46Plaster11168.02.111.19-3.31104.52.341.12-4.0463.61.810.66-3.59Magnesium oxide110.33.010.10-11.3800.200-inf10.16.430.21-24.36Multiple pollutant categories195.41.550.69-2.8162.91.910.69-3.8432.51.150.24-2.85??Skin cancer?Cement87161172.41.120.90-1.378691.61.100.83-1.417580.81.100.81-1.46Lime482624.81.130.71-1.661513.41.240.67-1.991111.41.030.50-1.79Plaster1144.30.870.23-1.9922.40.930.12-2.6621.90.820.11-2.37Magnesium oxide100.300-inf00.200-inf00.100-infMultiple pollutant categories103.500-inf01.800-inf01.700-inf??Breast cancer?Cement8723612377.40.990.92-1.06Lime48342308.01.110.97-1.27Plaster116957.61.280.96-1.65Magnesium oxide112.40.470.02-1.75Multiple pollutant categories15742.41.240.86-1.73??Vulvar and vaginal cancer?Cement87125130.20.990.79-1.22Lime482917.71.651.08-2.36Plaster1113.00.310.01-1.18Magnesium oxide100.200-infMultiple pollutant categories142.51.680.45-3.83??Uterine cancer?Cement87753733.90.990.89-1.10Lime4811195.91.170.93-1.43Plaster112217.51.350.82-2.03Magnesium oxide110.71.590.05-6.01Multiple pollutant categories11313.21.030.51-1.77??Ovarian cancer?Cement87680738.60.960.87-1.06Lime489195.41.000.79-1.23Plaster112217.41.410.87-2.09Magnesium oxide100.700-infMultiple pollutant categories1613.10.480.17-0.95??Prostate cancer?Cement8718772004.70.970.90-1.04?Lime48311298.41.040.90-1.19?Plaster114949.50.970.70-1.30?Magnesium oxide113.60.260.01-1.00?Multiple pollutant categories14139.91.000.66-1.43???Testicular cancer?Cement871218.20.740.36-1.30?Lime4822.50.950.12-2.71?Plaster1120.64.220.53-12.43?Magnesium oxide100.000-inf?Multiple pollutant categories100.300-inf???Bladder cancer?Cement8717521555.91.111.02-1.2014711280.31.141.05-1.25281275.60.980.84-1.13Lime48214220.60.990.84-1.16185182.81.050.88-1.252937.80.760.50-1.08Plaster113738.20.980.66-1.373031.90.970.63-1.4176.31.130.45-2.14Magnesium oxide102.300-inf02.000-inf00.300-infMultiple pollutant categories12729.50.920.54-1.421924.10.820.45-1.3485.41.380.58-2.58??Renal cancer?Cement87722681.31.000.90-1.11482450.51.010.89-1.13240230.81.020.86-1.20Lime4812592.91.331.08-1.617962.31.260.97-1.584630.71.541.10-2.06Plaster111116.90.730.40-1.24811.50.770.33-1.4135.40.600.13-1.47Magnesium oxide100.900-inf00.600-inf00.200-infMultiple pollutant categories11212.40.910.45-1.5758.10.580.19-1.2374.31.660.64-3.23??Brain cancer?Cement87961938.11.020.93-1.11545520.61.040.93-1.16416417.50.990.87-1.12Lime48149123.41.251.03-1.487869.61.160.90-1.457153.81.371.05-1.74Plaster112724.91.150.74-1.651714.51.240.71-1.931010.41.010.48-1.76Magnesium oxide121.01.720.22-4.8610.61.590.05-6.0110.42.030.07-7.66Multiple pollutant categories11916.31.180.67-1.8599.01.020.45-1.85107.31.380.64-2.45??Cancer of other parts of nervous system?Cement874232.61.430.92-2.101816.21.170.65-1.892416.41.700.91-2.86Lime4824.40.550.07-1.5712.20.480.02-1.8012.10.670.02-2.55Plaster1110.91.620.06-6.2300.500-inf10.44.060.15-15.98Magnesium oxide100.000-inf00.000-inf00.000-infMultiple pollutant categories110.62.220.09-8.7100.300-inf10.34.200.15-17.60??Thryroid cancer?Cement87111106.81.020.80-1.274035.91.090.74-1.527170.90.980.73-1.29Lime481714.41.190.68-1.8644.90.800.22-1.77139.51.410.73-2.33Plaster1122.50.800.10-2.2710.91.010.03-3.8311.60.640.02-2.40Magnesium oxide100.100-inf00.000-inf00.100-infMultiple pollutant categories112.00.500.02-1.8600.600-inf11.30.730.03-2.78??Ill-defined tumors?Cement8726292367.51.081.01-1.1515301319.01.121.03-1.2110991048.51.030.94-1.12Lime48335324.31.020.89-1.17209183.41.180.99-1.38126140.90.860.70-1.04Plaster116758.21.150.85-1.493733.81.180.80-1.663024.41.180.78-1.68Magnesium oxide113.00.430.01-1.6101.900-inf11.20.970.03-3.64Multiple pollutant categories14643.91.060.70-1.522624.01.090.64-1.682019.81.060.61-1.66??Non-Hodgkin's lymphoma?Cement871005926.51.030.93-1.13530483.21.050.92-1.19475443.30.970.85-1.10Lime48115125.50.850.68-1.046766.70.930.70-1.214858.70.780.56-1.04Plaster111823.40.820.47-1.27813.00.670.28-1.231010.41.020.48-1.79Magnesium oxide101.100-inf00.600-inf00.500-infMultiple pollutant categories11216.80.640.31-1.1278.70.740.28-1.4758.10.540.17-1.16??Hodgkin's lymphoma?Cement879997.60.990.78-1.244655.10.820.58-1.115342.51.240.88-1.67Lime481513.21.090.60-1.7497.51.150.52-2.0565.61.050.38-2.08Plaster1132.81.070.22-2.6121.61.200.15-3.3911.10.880.03-3.32Magnesium oxide100.100-inf00.100-inf00.000-infMultiple pollutant categories131.71.570.32-3.8931.02.760.57-6.8400.800-inf??Myeloma?Cement87655588.41.070.96-1.18324288.01.130.98-1.29331300.41.040.90-1.19Lime488580.51.030.81-1.293840.50.930.65-1.264740.01.160.84-1.54Plaster111113.90.760.37-1.2877.20.960.38-1.8246.80.570.16-1.27Magnesium oxide110.71.460.05-5.4900.400-inf10.33.180.10-12.02Multiple pollutant categories11710.91.480.83-2.3595.31.630.73-2.9585.61.380.58-2.57??Leukemia?Cement9012251151.11.050.97-1.13685637.11.070.97-1.17540514.01.050.94-1.16Lime52177160.41.130.95-1.3210090.81.130.91-1.387769.51.100.86-1.38Plaster112429.60.810.51-1.191517.10.930.51-1.47912.60.690.32-1.22Magnesium oxide121.41.600.20-4.5120.92.500.32-7.0800.500-infMultiple pollutant categories13221.11.380.91-1.98?1311.71.060.55-1.75?199.51.801.06-2.77aNumber of towns situated at ≤5 km from installations for the production of cement, lime, plaster, and magnesium oxide as a whole.bObserved deaths.cExpected deaths.dRRs adjusted for population size, percentages of illiteracy, farmers and unemployed persons, average persons per household, and mean incomee95% credible interval.fSum of the 33 types of cancer analyzed.Supplementary data, Table S5.????Pollutants released in the last twelve yearsaPRTR codeIndustrial activityProvinceMunicipalityAirWater141CementVALENCIASaguntoMethane, CO, CO2, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, naphthalene, anthracene, fluorine, PCBs?142CementCORDOBACórdobaCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, total suspended particles, vanadium, manganese, cobalt, total organic carbon, ammonia, fluorine, antimony, hydrogen cyanide, thallium?143CementTOLEDOVillaluenga de la SagraMethane, CO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, benzene, PAHs, chlorine, PM10, total suspended particles, fluorineNitrogen, phosphorus, total organic carbon144CementBARCELONAMontcada i ReixacCO, CO2, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, total suspended particles, naphthalene, anthracene, vanadium, manganese, cobalt, total organic carbon, ammonia, fluorine, PCBs, antimony, hydrogen cyanide, di-(2-ethyl hexyl) phthalate, thallium?145CementHUELVANieblaCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, total suspended particles, naphthalene, anthracene, vanadium, manganese, cobalt, total organic carbon, ammonia, fluorine, PCBs, antimony, hydrogen cyanide, di-(2-ethyl hexyl) phthalate, thallium?296CementBARCELONASant Vicen? dels HortsCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, total suspended particles, naphthalene, anthracene, vanadium, manganese, cobalt, total organic carbon, ammonia, fluorine, PCBs, antimony, hydrogen cyanide, di-(2-ethyl hexyl) phthalate, thalliumCopper, zinc, nitrogen, phosphorus, phenols, total organic carbon, chlorides1082CementHUELVAPalos de la FronteraTotal suspended particles?1494CementTOLEDOYelesMethane, CO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, PAHs, chlorine, total suspended particles, fluorineNitrogen, phosphorus, total organic carbon1496CementLUGOSarriaCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, naphthalene, anthracene, ammonia, fluorine, PCBs, hydrogen cyanide, di-(2-ethyl hexyl) phthalate,?1497CementLEONVilladecanesCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, total suspended particles, naphthalene, anthracene, vanadium, manganese, cobalt, total organic carbon, ammonia, fluorine, PCBs, antimony, hydrogen cyanide, di-(2-ethyl hexyl) phthalate, thallium?1512CementMALAGAMálagaCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, total suspended particles, naphthalene, anthracene, vanadium, manganese, cobalt, ammonia, fluorine, PCBs, antimony, hydrogen cyanide, di-(2-ethyl hexyl) phthalate, thallium?1570CementCADIZJerez de la FronteraCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, dioxins and furans, benzene, PAHs, PM10, total suspended particles, naphthalene, manganese, total organic carbon, ammonia, hydrogen cyanide, di-(2-ethyl hexyl) phthalate, ?1572CementALMERIAGádorCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, total suspended particles, naphthalene, anthracene, vanadium, manganese, cobalt, ammonia, fluorine, PCBs, antimony, hydrogen cyanide, di-(2-ethyl hexyl) phthalate, thallium?1573CementALMERIACarbonerasCO, CO2, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, naphthalene, anthracene, vanadium, hydrogen cyanide, di-(2-ethyl hexyl) phthalateLead, zinc, nitrogen, phosphorus, total organic carbon, fluorides1574CementMURCIALorcaCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, total suspended particles, naphthalene, anthracene, vanadium, manganese, cobalt, total organic carbon, ammonia, fluorine, PCBs, antimony, hydrogen cyanide, di-(2-ethyl hexyl) phthalate, thallium?1757CementSEVILLAAlcalá de GuadaíraCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, cadmium, chromium, dioxins and furans, benzene, PAHs, chlorine, PM10, total suspended particles, naphthalene, anthracene, ammonia, fluorine, PCBs?1758CementPALENCIAVenta de Ba?osCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, benzene, PAHs, chlorine, PM10, naphthalene, ammonia, fluorine, hydrogen cyanide, di-(2-ethyl hexyl) phthalateTotal organic carbon1759CementMADRIDMorata de Taju?aCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, total suspended particles, naphthalene, ammonia, vanadium, manganese, cobalt, total organic carbon, fluorine, PCBs, hydrogen cyanide, thallium?1760CementNAVARREOlaztiMethane, CO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, lead, zinc, benzene, PAHs, chlorine, PM10, naphthalene, ammonia, manganese, cobalt, PCBs, antimony, hydrogen cyanide, thalliumCODc1914CementASTURIASOviedoCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, naphthalene, ammonia, fluorine, hydrogen cyanide, di-(2-ethyl hexyl) phthalate?1915CementASTURIASCarre?oCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, naphthalene, anthracene, ammonia, fluorine, PCBs, hydrogen cyanide, di-(2-ethyl hexyl) phthalateTotal organic carbon, CODc1916CementLEONLa RoblaCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, naphthalene, anthracene, ammonia, fluorine, PCBs, hydrogen cyanide, di-(2-ethyl hexyl) phthalate?2072CementCANTABRIAValdeoleaCO, CO2, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, total suspended particles, naphthalene, anthracene, vanadium, manganese, cobalt, total organic carbon, ammonia, fluorine, PCBs, antimony, hydrogen cyanide, thallium?2578CementTARRAGONAAlcanarCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, chlorine, PM10, total suspended particles, naphthalene, ammonia, fluorine, PCBs, hydrogen cyanide, di-(2-ethyl hexyl) phthalateNitrogen, phosphorus, CODc2580CementVALENCIABu?olMethane, CO, CO2, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, naphthalene, ammonia, anthracene, fluorine, PCBs, di-(2-ethyl hexyl) phthalate?2581CementBARCELONAVilanova i La GeltrúCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, total suspended particles, naphthalene, anthracene, vanadium, manganese, cobalt, total organic carbon, ammonia, fluorine, antimony, di-(2-ethyl hexyl) phthalate, thallium?2582CementBARCELONASant Feliu de LlobregatMethane, CO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, total suspended particles, naphthalene, anthracene, vanadium, manganese, cobalt, total organic carbon, ammonia, fluorine, PCBs, antimony, hydrogen cyanide, di-(2-ethyl hexyl) phthalate, thallium?2583CementTOLEDOYepesMethane, CO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, benzene, PAHs, chlorine, PM10, total suspended particles, fluorineTotal organic carbon2584CementBALEARIC ISLANDSLlosetaCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, total suspended particles, naphthalene, anthracene, vanadium, manganese, cobalt, total organic carbon, ammonia, fluorine, PCBs, antimony, hydrogen cyanide, di-(2-ethyl hexyl) phthalate, thallium?2585CementZARAGOZAMorata de JalónCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, benzene, PAHs, chlorine, PM10, total suspended particles, naphthalene, anthracene, vanadium, manganese, cobalt, ammonia, fluorine, PCBs, antimony, hydrogen cyanide, di-(2-ethyl hexyl) phthalate, thalliumCODc2586CementALICANTESant Vicent del RaspeigMethane, CO, CO2, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, naphthalene, anthracene, ammonia, fluorine, PCBs, di-(2-ethyl hexyl) phthalate?2898CementTERUELSanta EulaliaPM10?3036CementBARCELONASanta Margarida i Els MonjosCO, CO2, NMVOCb, NO2, SO2, cadmium, copper, mercury, nickel, lead, zinc, benzene, chlorine, PM10, manganese, cobalt, ammonia, PCBs, hydrogen cyanide?3037CementBARCELONASitgesCO, CO2, NMVOCb, NO2, SO2, cadmium, chromium, copper, mercury, nickel, lead, zinc, benzene, chlorine, PM10, naphthalene, anthracene, vanadium, manganese, ammonia, PCBs, thallium?3581CementMALAGAAntequeraCO, NO2, SO2, PM10?3686CementVIZCAYAArrigorriagaCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, naphthalene, anthracene, ammonia, fluorine, PCBs, hydrogen cyanide, di-(2-ethyl hexyl) phthalate?3687CementGUIPUZCOASan SebastiánCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, naphthalene, anthracene, ammonia, fluorine, PCBs, hydrogen cyanide, di-(2-ethyl hexyl) phthalate?3718CementVIZCAYALemoaCO, CO2, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, chlorine, PM10, ammonia, fluorine, PCBs?4861CementGERONABoadella i Les EscaulesCO, CO2, NO2, SO2, total suspended particlesNitrogen, phosphorus, CODc6816CementSANTA CRUZ DE TENERIFESanta Cruz de TenerifeCO, CO2, NO2, SO2, PM10CODc6828CementLAS PALMASSan Bartolomé de TirajanaCO, CO2, NO2, chromium, zinc, chlorine, PM10Arsenic, chromium, nickel, lead7662CementVALENCIARiba-Roja de TúriaMethane, CO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, PM10?7946CementMALAGAMálagaTotal suspended particles?220LimeBARCELONAOlesa de BonesvallsCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, naphthalene, anthracene, ammonia, fluorine, di-(2-ethyl hexyl) phthalateTotal organic carbon306LimeBARCELONAPacs del PenedèsCO, CO2, NO2, SO2, PM10, total suspended particlesCODc645LimeCASTELLONChilchesMethane, CO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, ammonia, fluorine, dichloromethane?814LimeGERONAGeronaMethane, CO, CO2, nitrous oxide, NMVOCb, NO2, SO2?822LimeGERONAArgelaguerCO2Nitrogen, phosphorus984LimeGRANADAHuétor de SantillánCO, CO2, NMVOCb, NO2, SO2, nickel, zinc, PM10?1662LimeMADRIDArganda del ReyCO, CO2, NO2, SO2, cadmium, mercury, PM10, total suspended particles?1668LimeMADRIDColmenar de OrejaCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, total suspended particles, naphthalene, anthracene, ammonia, fluorine, di-(2-ethyl hexyl) phthalate?1944LimeASTURIASLlaneraCO, CO2, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, fluorine, PCBs, di-(2-ethyl hexyl) phthalate?2329LimeSEVILLAEstepaCO, CO2, NMVOCb, NO2, SO2, arsenic, cadmium, mercury, lead, zinc, benzene, PM10, total suspended particles, ammonia?2344LimeSEVILLAMorón de la FronteraCO, CO2, nitrous oxide, NMVOCb, NO2?2710LimeCANTABRIACastro-UrdialesCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, chromium, copper, lead, zinc, dioxins and furans, PAHs, PM10?3563LimeNAVARRETiebas-Muruarte de RetaMethane, CO, CO2, nitrous oxide, NMVOCb, NO2, SO2, PM10?3564LimeSEVILLAEstepaCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, nickel, lead, zinc, dioxins and furans, benzene, PAHs, chlorine, PM10, fluorine?3664LimeGUIPUZCOAAltzoCO, CO2, NO2, SO2, PM10?4095LimeZARAGOZAPuebla de AlbortónCO, CO2, nitrous oxide, NMVOCb, NO2, SO2, arsenic, cadmium, chromium, copper, mercury, lead, zinc, benzene, PAHs, PM10, naphthalene, ammonia, di-(2-ethyl hexyl) phthalate?4515LimeZARAGOZAMorésMethane, CO, CO2, NMVOCb, NO2, SO2, PM10, total suspendes particles?5218LimeSEVILLAPedreraCO, CO2, NMVOCb, NO2, SO2, PAHs, PM10?6562PlasterMADRIDValdemoroCO, CO2, NO2, total suspended particles?6581PlasterBURGOSValle de OcaCO, CO2, NO2, SO2, PM10?7034PlasterMADRIDSan Martín de la VegaMethane, CO, NO2, SO2, PM10?7484PlasterGERONABeudaCO, CO2, NO2, SO2, total suspended particles?1558Magnesium oxideLUGOO IncioCO, CO2, NO2, SO2, PM10?1763Magnesium oxideNAVARREEsteríbarCO, CO2, NO2, SO2, PM10? aPollutants released in the period 2001-2012 and included in the IPCC database.bNon-methane organic hemical oxygen demand.Supplementary data, Table S6.?Releases to air (IPPC, 2009) (kg/year)PRTR CodeA1aA2A3A4A5A6A7A8A9A10A11A12A13A14A15A16A17A18A19A20A21A22A23A24A25A26A27A28A29A30A31A32A33A34A35TOTAL1418??91937??566?1617300277270000001560.00024?25331018900007717?520000158000012000?0.0000345????76731023837142?11700101096459261311980514378007463000000362109553050006526021801480000595066100.0000267519464859076143?50.01226141920158730000001283417300504000449420020300003000041187558791014438498116710.15704291350.20.4263060.2284374000410.00010.40.1569449330.412215617132161717960.0000112330.23628566900614548510447003188009523101727400123370000001300.0001797618500034838202460068000029100324000.00001203344453380131402200.001301247254307593651263016030270.0252519950443142322909118007.6E-0763563095358296102499310112055955096280677642180534359751930003830.00032332017214415110022112196742141578528418300.0000159910111132979813863306?1128404907372691718247064616461113063536645?2560.34260.1389013854244790000025590.617112600393266003740022900.0001213947984819814?6351365882638643424547136951446516822?7236808572368085984?202018600000112005880272003550186498501082?4714711494?0.833270942952830000001301138601990002255755900090500.712283774856149649400477431055548151001335300000020.000188662100037842007500872000265000.000022238503545574161497615500771280549900174422021350100225840000002380.00021451211437000621469805920111000024500272000.0000337663782585733513151276617713105178430021451200226000000002430.00020.7131114700006314713046700101000044700497000.00003376647846026864861558?116000000650007200001530001169380001570?145002184700020025470063340000003494770003260066200010400115003.0E-06335228225157251320055475127247013136024480000007100.00011064832743000452508012900113000028300283007.6E-0783461604499658691573645505040.716665002387356900000040713842150005912400086100080200.00001160465702213031574126700332440.714500338640.50.595700.81210000001340.000032833228000120.513303170043100037400416000.000030.81122161218231621662?967450008760050700304001880030209693552016680.0000490.1130.11230.12670.421410000.80.00040.126211352015613033369912.2E-080.20.10.1216459817570.275831904970137300000003763.4E-06105373000100176001610000210000.000017320311121758?11900897911332690143840024330000001831191000017546001410000487011334364338431759?5551253797017714100435576049880000001090.000112221410000528518085900182000028500316002.0E-0611273129914103401760?972481900084850000000.0111153201135007818000946000436000153114865479751763?3270000006870064000002070000384003355771001914738008175424529030346002046200000011049410200003243940447000674000656000.000011799166464252090191571580081300517642721350800225760000002420.0002147111060000631470706890001870000803000.000033764835797794341916921000101730723557001867700307540000003220.00021961517800008419943016200002550000167000.0000349851117600734491944?58928283558300000612370.286500448866605630513458400660207251728885234630013915901383990044680000001460.00011151012344000049771500063000016800235000.00001583654729147222329?960.0230.0031080000228000000.0437800850001890665000.10.5240712902344?282001720000004950056801400001722233802578?622812803930844187271872710518904791022.0E-061913194151125123343550242733649063834710.0000427595010558249402580563424145011174000183260000003650.00012432630126000051123460001050000965000.00002308832893153925810.21160.20.230.21400.10.816590.425344000850.40.411891420.523121893335997348538738.0E-0720.220.232572737725820.0032210.40.4690.32151112650.20.8314411363210001390.0000190.80.7132919813840.943834469202422325332531.2E-0620.430.551367703312583?140.0133880151130878200000012302291020057500085026401010000304007043783634722258424580223762425005112400.74148006166000000700.0001434352100018420502910005830009710379000.00001112192241675084252585699920548230.51797240352440034790000001922831612460000933135008158880002210015400127310113048244322425869919871813200307020000006640.00021411329075500085192540001250000359000.0000150967043126022710?4713.418896440000.02932526887534808601.1E-0697897985372898?124012403036?44041615353053611402658974549260.002140.948527938351471772243102590466590426577430370.0216372890.857542405576351999400.01515319376816418715581926577659735356395044453563?3821440000003822650007641180010300089801443903083564?50.20.116001021000231480000004910.0040.42620021260834049400489000.00001371481572423581?123078556431628953664?16552281436682936860.0289504731100248276677491140.00010.141831638362740182521071262259189750.00001153647338762036870.0000002726110.36217442334750.00014.1E-080.311391790.0001343606555221624566129061.5E-06195034418643718?1208261612161842904200030.000017306373367614876380623640.000024644329608694095?4574716771420019954000000.02816900076673015600104000179001047957287464515?9250353000002432810048642200709000360892794861?2108680308008300222849221505005218?477443000000.001406000113026706410447166876562?24236000637001860082200244005006581?2040000014300765004390016800205515006816?234000043126308190683023580816828?27935170156322257753711577417353867034?22102595710.127347484?73206539143177912519271873685837662?0.020.020.022030.0110700000.02241790.02135211080122006.2E-090.10.0310842207946?186186TOTAL1662421816919519911127342185295510945149538208645553019254716728811922059201277581244396004914073521421421590603342485530108462114024220.00059636910521366195619362576996aA1: Anthracene. A2: Ammonia. A3: Antimony. A4: Arsenic and compounds. A5: Benzene. A6: Cadmium and compounds. A7: Total organic carbon. A8: Hydrogen cyanide. A9: Chlorine and inorganic compounds. A10: Cobalt. A11: Copper and compounds. A12: Non-methane volatile organic compounds. A13: Chromium and compounds. A14: CO2. A15: Fluorine and inorganic compounds. A16: PCBs. A17: PAHs. A18: Manganese. A19: Mercury and compounds. A20: Methane. A21: CO. A22: Naphthalene. A23: Nickel and compounds. A24: Nitrous oxide. A25: SOx/SO2. A26: NOx/NO2. A27: PM10. A28: Total suspended particles. A29: Dioxins and furans. A30: Lead and compounds. A31: Thallium. A32: Di-(2-ethyl hexyl) phthalate. A33: Dichloromethane. A34: Vanadium. A35: Zinc and compounds.Supplementary data, Table S7.?Releases to water (IPPC 2009) (kg/year)PRTR CodeW1aW2W3W4W5W6W7W8W9W10W11W12W13TOTAL141?????????????01420143811311521014401450220636329611043430.40.4845980.851363063434645081408229324198401082014941621230149601497015120155801570015720157312957692340.628315740166201668017570175867567517590176012011201176301914019157172150286719160194402072023290234402578788436614229672258002581025820258351512584025852662662586027100289803036030370356303564035810366403686036870371804095045150486140.10.34521806562065810681637037068280.0317670.0420.040.03176970340748407662079460TOTAL0.03401443430.40.04115042575430.0422024122672 aW1: Arsenic and compounds. W2: Total organic carbon. W3: Chlorides. W4: Copper and compounds. W5: Chromium and compounds. W6: Chemical oxygen demand. W7: Phenols. W8: Fluorides. W9: Total phosphorus. W10: Nickel and compounds. W11: Total nitrogen. W12: Lead and compounds. W13: Zinc and compounds.Supplementary data, Figure S1. ................
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