4. K. W. Chen, Y. Lai, Y.-C. Chiu, S. Steven, T. Besara, D ...



PUBLICATIONS AND PATENTSCENTER FOR ACTINIDE SCIENCE AND TECHNOLOGY 202089.J. M. Sperling, E. J. Warzecha, C. Celis-Barros, D.-C. Sergentu, X. Wang, B. E. Klamm, C. J. Windorff, A. N. Gaiser, F. D. White, D. A. Beery, A. T. Chemey, M. A. Whitefoot, B. N. Long, K. Hanson, E. Zurek, J. Autschbach, T. E. Albrecht-Schmitt, “Compression of Certain Curium Coordination Complexes Enhances Covalency,” Nature 2020 (in revision).88. B. E. Cole, T. Cheisson, R. F. Higgins, E. Nakamaru-Nagiso, B. C. Manor, P. J. Carroll, E. J. Schelter, “Redox-Driven Chelation and Kinetic Separation of Select Rare Earths Using a Tripodal Nitroxide Proligand,” Inorganic Chemistry 2020, 59 (1), 172-178. DOI: 10.1021/acs. inorgchem.9b0097587.Y. Hao, P. Kegler, T. E. Albrecht-Schmitt, S. Wang, Q. Dong, E. V. Alekseev, “Two-Dimensional Uranyl Borates: From Conventional to Extreme Synthetic Conditions,” European Journal of Inorganic Chemistry, 2020, 407-416. DOI: 10.1002/ejic. 20190123986. T. Jian, X. Yu, D. Dan, T. Albrecht-Schmitt, J. Autschbach, J. Gibson, "Gas-Phase Com-plexes of Americium and Lanthanides with a Bis-Triazinyl Pyridine: Reactivity and Bonding of Archetypes for f-Element Separations," J. Phys. Chem. A 2020 (in press). DOI: org/10.1021/acs.jpca.0c0067585.J. J. M. Nelson, T. Cheisson, H. J. Rugh, M. R. Gau, P. J. Carroll, E. J. Schelter, “High-Throughput Screening for Discovery of Benchtop Separations Systems for Selected Rare Earth Elements,” Commun. Chem. 2020, 3, 7. DOI: org/10.1038/s42004-019-0253-x84. A. T. Chemey, J. M. Sperling, D. E. Hobart, T. E. Albrecht–Schmitt, “Structural Relationships and Absorption Spectroscopy of β-NH4UF5 and NH4Pu3F13,” Crystal Growth & Design 2020 (in revision).83.K. Hinz, D. Fellhauer, X. Gaona, M. Vespa, K. Dardenne, D. Schild, T. Yokosawa, M. A. Silver, D. T. Reed, T. E. Albrecht-Schmitt, M. Altmaier, H. Geckeis, “Interaction of Np(V) with Borate in Alkaline, Dilute-to-Concentrated, NaCl and MgCl2 Solutions,” Dalton Trans. 2020, 49, 1570-1581. DOI: 10.1039/C9DT04430B.82.C. J. Windorff, C. Celis-Barros, J. M. Sperling, B. E. Klamm, N. C. McKinnon, T. E. Albrecht-Schmitt, “Probing the Inverse Trans Influence in Americium and Lanthanide Tribromide Tris(Tricyclohexylphosphine Oxide),” Chemical Science, 2020, 11, 2770-2782. DOI: 10.1039/C9SC05268B81,J. M. Sperling; A. N. Gaiser; C. J. Windorff; B. E. Klamm, M. A. Whitefoot, A. T. Chemey, B. N. Long, J. Campbell, T. E. Albrecht-Schmitt, 2020, “Structural and Spectroscopic Investigation of Two Plutonium Mellitates,” Inorg. Chem. 2020, 59, 5, 3085-3090. DOI: 10.1021/acs.inorgchem.9b03432 80.Z.-H. Zhang, J.-H. Lan, L.-Y. Yuan, P.-P. Sheng, M.-Y. He, L.-R. Zheng, Q. Chen, Z.-F. Chai, J. K. Gibson, W.-Q. Shi, “Rational Construction of Porous Metal-Organic Frameworks for Uranium(VI) Extraction: The Strong Periodic Tendency with a Metal Node,” ACS Appl. Mater. Interfaces. 2020, March 10. DOI: 10.1021/acsami.0c02121 [Epub ahead of print]79.W. L. Nelson, A. T. Chemey, M. Hertz, E. Choi, D. E. Graf, S. Latturner, T. E. Albrecht-Schmitt, K. We, R. E. Baumbach, “Superconductivity in a Uranium Containing High Entropy Alloy,” Sci. Rep. 2020, 10, 4717. DOI: org/10.1038/s41598-020-61666-z201978. J. Yu, L. Yuan, S. Wang, J. Lan, L. Zheng, C. Xu, J. Chen, L. Wang, Z. Huang, W. Tao, Z. Liu, Z. Chai, J. K. Gibson, W. Shi, “Phosphonate-Decorated Covalent Organic Frame-works for Actinide Extraction: A Breakthrough Under Highly Acidic Conditions,” CCS Chemistry, 2019, 1, 286–295. DOI:10.31635/ccschem.019.20190005 77. A. T. Chemey, T. E. Albrecht-Schmitt, “Redetermination of the Crystal Structure of Tetra-Lithium Octa-Fluorido-Zirconate(IV), Li4ZrF8, from Single-Crystal X-ray Data,” Acta Crystallographica, Section E, Crystallographic Communications 2019, 75 (Part 2), 139–141. DOI: 10.1107/S205698901801819476. M. L. Marsh, F. D. White, D. S. Meeker, C. D. McKinley, D. Dan, C. Van Alstine, T. N. Poe, D. L. Gray, D. E. Hobart, T. E. Albrecht-Schmitt, “Electrochemical Studies of Selected Lanthanide and Californium Cryptates,” Inorganic Chemistry 2019, 58, 9602-9612. DOI: 10.1021/acs.inorgchem.9b0092075. C. A. P. Goodwin, J. Su, T. E. Albrecht Schmitt, E. R. Batista, A. V. Blake, W. J. Evans, A. J. Gaunt, S. A. Kozimor, N. Lichtenberger, B. L. Scott, P. Yang, “[Am(C5Me4H)3], an Organometallic Am(III) Complex,” Angewandte Chemie, Int. Ed. 2019, 58, 11695-11699. DOI: 10.1002/anie.20190522574. J. Zhuang, L. Abella, D. -C. Sergentu, Y. -Rong Yao, M. Jin, W. Yang, X. Zang, X. Li, D. Zhang, Y. Zhao, X. Li, S. Wang, L. Echegoyen, J. Autschbach, N. Chen, “Diuranium(IV) Carbide Cluster U2C2 Stabilized Inside Fullerene Cages” J. Am. Chem. Soc. 2019, 141, 51, 20249-2026. DOI:10.1021/jacs.9b10247 73. A. T. Chemey, C. Celis-Barros, J. M. Sperling, D. Paez-Hernandez, T. E. Albrecht-Schmitt, “Structure, Spectroscopy, and Theoretical Analysis of Zero- and Three-Dimensional Lithium Plutonium Fluorides: Li4PuF8 and LiPuF5,” Inorg. Chem. 2019, 58 (21), 14790-14799. DOI: 10.1021/acs.inorgchem.9b0246672. D. L. Clark, D. E. Hobart, “Discovery of the Transuranium Elements Inspired Rearrange-ment of the Periodic Table and the Approach for Finding New Elements,”, in Structure and Bonding - The Periodic Table 1: Historical Development and Essential Features 2019, Springer, Berlin, Heidelberg, DOI: 10.1007/430_2019_4672; Los Alamos National Laboratory report LA-UR-19-26646. 71. D. Dan, C. Celis-Barros, F. D. White, J. M. Sperling, T. E. Albrecht-Schmitt, “Origin of Selectivity of a Trazinyl Ligand for Americium(III) over Neodymium(III),” Chem. Eur. J. 2019, 25, 3248-52. DOI: 10.1002/chem.201806070.70. K. Huang, W. L. Nelson, A. T. Chemey, T. Albrecht-Schmitt, and R. E. Baumbach, “A Novel Cage for Actinides: A6W4Al43 (A = U and Pu),” J. Phys. Condensed Matter 2019, 31, 165601. DOI: 10.1088/1361-648X/aafe9e69. L. Wang, H. Song, L. Yuan, Z. Li, P. Zhang, J. K. Gibson, L. Zheng, H. Wang, Z. Chai, W. Shi, "Effective Removal of Anionic Re(VII) by Surface-Modified Ti2CTx MXene Nanocomposites: Implications for Tc(VII) Sequestration," Envir. Sci. Technol. 2019, 53, 3739–3747 DOI: 10.1021/acs.est.8b0708368. L. Mei, F. Li, J. Lan, C. Wang, C. Xu, H. Deng, Q. Wu, K. Hu, L. Wang, Z. Chai, J. Chen, J. K. Gibson, W. Shi, “Anion-Adaptive Crystalline Cationic Material for 99TcO4? Trapping,” Nature Comm. 2019, 10, Article?number:?1532 DOI: 10.1038/s41467-019-09504-367. I. Lehman-Andino, J. Su, K. E. Papathanasiou, T. M. Eaton, J. Jian, D. Dan, T. E. Albrecht-Schmitt, C. J. Dares, E. R. Batista, P. Yang, J. K. Gibson and K. Kavallieratos, “Soft-donor Dipicolinamide Derivatives for Selective Actinide(III)/ Lanthanide(III) Separation: The Role of S- vs. O-donor Sites,” Chem. Commun. 2019, 55, 2441, DOI: 10.1039/C8CC07683A.66. C. A. P. Goodwin,?J. Su, T. E. Albrecht-Schmitt,?A. V. Blake, E. R. Batista, S. R. Daly, S. Dehnen, W. J. Evans, A. J. Gaunt, S. A. Kozimor,?N. Lichtenberger, B. L. Scott, P. Yang, “[Am(C5Me4H)3]: An Organometallic Americium Complex” ?Angewandte Chemie, International Edition 2019, 131, 11821-11825 DOI: 0.1002/anie.20190522565. K. C. Mullane, P. Hrobárik, T. Cheisson, B. C. Manor, P. J. Carroll, and E. J. Schelter, “13C NMR Shifts as an Indicator of U–C Bond Covalency in Uranium(VI) Acetylide Complexes: An Experimental and Computational Study”, Inorg. Chem. 2019, 58 (7), pp 4152–4163. DOI: 10.1021/acs.inorgchem.8b03175.64. V. Proust, R. Jeannin, F. D. White, T. E. Albrecht-Schmitt, “Tailored Perovskite Waste Forms for Plutonium Trapping,” Inorg. Chem. 2019, 58 (5), pp 3026–303 DOI: 10.1021/acs. inorgchem. 8b02832.63. F. D. White, C. Celis-Barros, J. Rankin, E. Solís-Céspedes, D. Dan, A. N. Gaiser, Y. Zhou, J. Colangelo, D. Páez-Hernández, R. Arratia-Pérez?, T. E. Albrecht-Schmitt, ”Molecular and Electronic Structure, and Hydrolytic Reactivity of a Samarium(II) Crown Ether Complex,” Inorg. Chem. 2019, 58(5), 3457–3465, DOI: 10.1021/acs.inorgchem. 8b03566.62. V. Ovidiu Garlea, L. D. Sanjeewa, M. A. McGuire, C. D. Batista, A. M. Samarakoon, D. Graf, B. Winn, F. Ye, C. Hoffmann, J. W. Kolis, “Exotic Magnetic Field-Induced Spin-Super-structures in a Mixed Honeycomb-Triangular Lattice System,” Phys. Rev X 2019, 9, (1) 011038, DOI: org/10.1103/PhysRevX.9.01103861. A. T. Chemey, T. E. Albrecht-Schmitt, “Redetermination of the Crystal Structure of Tetra? Lithium octa?fluorido?zirconate(IV), Li4ZrF8, from Single-Crystal X-ray Data,” Acta Cryst. 2019, E75, 139-141, DOI: 10.1107/S205698901801819460. T. Cheisson, E. J. Schelter, “Rare Earth Elements: Mendeleev’s Bane, Modern Marvels,” Science 2019, 363, (6426), 489-493. DOI: 10.1126/science.aau762859. T. Cheisson, B. E. Cole, B. C. Manor, P. J. Carroll, E. J. Schelter, “Phosphoryl-Ligand Adducts of Rare Earth-TriNOx Complexes: Systematic Studies and Implications for Separations Chemistry,” ACS Sustainable Chem. Eng. 2019, 7(5), 4993–5001. DOI: 10.1021/acssuschemeng.8b0563858. T. Cheisson, K. D. Kersey, N. Mahieu, A. McSkimming, M. R. Gau, P. J. Carroll, E. J. Schelter, “Multiple Bonding in Lanthanides and Actinides: Direct Comparison of Covalency in Thorium(IV)- and Cerium(IV)-Imido Complexes,” J. Am. Chem. Soc. 2019, 141 (23), 9185-9190.adducts of rare earth DOI: 10.1021/jacs.9b0406157. T. Cheisson, J. Jian, J. Su, T. M. Eaton, M. R. Gau, P. J. Carroll, E. R. Batista, P. Yang, J. K. Gibson, E. J. Schelter, “Halide Anion Discrimination by a Tripodal Hydroxylamine Ligand in Gas and Condensed Phases,” Phys. Chem. Chem. Phys. 2019, 21, 19868-19878, DOI: 10.1039/C9CP03764K 56. J. Lan, C. Wang, Q. Wu, Z. Chai, J. K. Gibson, W. Shi, “Modification of a Carbon Nanobelt with Actinides Th–Am: A Density Functional Theory Study,” J. Phys. Chem. A 2019, 123 (23), 4900-4907, DOI: 10.1021/acs.jpca.9b0285355. A. P. Dioguardi, H. Yasuoka, S. M. Thomas, H. Sakai, S. K. Cary, S. A. Kozimor, T. E. Albrecht-Schmitt, H. C. Choi, J.-X. Zhu, J. D. Thompson, E. D. Bauer, F. Ronning, “239Pu Nuclear Magnetic Resonance in the Candidate Topological Insulator PuB4,” Phys. Rev. B. 2019, 035104, DOI: 10.1103/PhysRevB.99.035104 54. H. Deng, Z. Li, X. Wang, L. Wang, K. Liu, L. Yuan, Z. Chang, J. K. Gibson, L. Zheng, Z. Chai, W. Shi, “Efficient Photocatalytic Reduction of Aqueous Perrhenate and Pertechnetate,” Environ. Sci. Technol. 2019, 53 (18), 10917-10925, DOI: 10.1021/ acs.est.9b0319953. R. R. Li, A. E. DePrince III, "The Role of Orbital Angular Momentum Constraints in the Variational Optimization of the Two-electron Reduced-density Matrix," Phys. Rev. A 2019, 100, 032509, DOI: 10.1103/PhysRevA.100.03250952. B. E. Klamm, C. J. Windorff, C. Celis-Barros, M. L. Marsh, T. E. Albrecht-Schmitt, “Synthesis, Spectroscopy, and Theoretical Details of Uranyl Schiff-Base Coordination Complexes,” Inorg. Chem. 2020, 59, 1, 23-31. DOI: org/10.1021/acs.inorgchem.9b0047751. A. S. Jayasinghe, Y. Lai, R. Baumbach, S. E. Latturner, “U1.33T4Al8Si2 (T = Ni, Co): Complex Uranium Silicides Grown from Aluminum/Gallium Flux Mixtures,” Inorg. Chem. 2019, 58 (18) 12209-12217, DOI: 10.1021/acs.inorgchem.9b0162750. S. Hu, J. Jian, J. Li, J. K. Gibson, “Destruction of the Uranyl Moiety in a U(V) “Cation–Cation” Interaction,” Inorg. Chem. 2019, 58 (15) 10148-10159, DOI: 10.1021/acs. inorgchem.9b0126549. V. O. Garlea, L. D. Sanjeewa, M. A. McGuire, C. D. Batista, A. M. Samarakoon, D. Graf, B. Winn, F. Ye, C. Hoffmann, J. W. Kolis, “Exotic Magnetic Field-Induced Spin-Superstructures in a Mixed Honeycomb-Triangular Lattice System,” Phys. Rev. X. 2019, 9, 011038, DOI: 10.1103/PhysRevX.9.01103848. J. N. Cross, T. Lee, C. Kang, Y. Yao, S. K. Cary, J. T. Stritzinger, M. J. Polinski, C. D. McKinley, T. E. Albrecht Schmitt, N. Lanata, “Origins of the Odd Optical Observables in Plutonium and Americium Tungstates,” Chem. Sci. 2019, 10, 6508-6518, DOI: 10.1039/ C9SC01174A; Press Release by Chemistry World: news/curious-colours-expose-f-electron-covalency-effects/3010564.article.47. K. Wei, J. N. Neu, Y. Lai, K.-W. Chen, D. Hobbis, G. S. Nolas, D. E. Graf, T. M. Siegrist, R. E. Baumbach, “Enhanced Thermoelectric Properties of Kagome Heavy-Fermion Compounds YbT2Zn20 (T = Co, Rh, Ir) at Low Temperatures,” NPJ Quantum Materials 2019, 5 (5), 1-7, DOI: 10.1126/sciadv.aaw618346. K. Huang, K.-W. Chen, A. Gallagher, Y. Lai, L. Nelson, D. Graf, and R. Baumbach, “Instability of the f-electron State in URu2Si2-xPx Probed Using High Magnetic Fields,” Phys. Rev. B 2019, 99 (23), 235146, DOI: 10.1103/PhysRevB.99.235146201845. Z. E. Brubaker, R. L. Stillwell, P. Chow, Y. Xiao, C. Kenney-Benson, R. Ferry, D. Popov, S. B. Donald, P. S?derlind, D. J. Campbell, J. Paglione, K. Huang, R. E. Baumbach, R. J. Zieve, J. R. Jeffries, “Pressure Dependent Intermediate Valence Behavior in YbNiGa4 and YbNiIn4,” Phys. Rev. B 2018, 98, 214115. DOI:10.1103/PhysRevB.98.214115.44. A. T. Chemey, J. M. Sperling, T. E. Albrecht-Schmitt, “Expanding Pentafluorouranates: Hydrothermal Synthesis and Characterization of β-NaUF5 and β-NaUF5·H2O,” RSC Advances 2018, 8, 28642-28648. DOI: 10.1039/c8ra05780j43. J. Li, X. Dai, L. Zhu, C. Xu, D. Zhang, M. Silver, P. Li, L. Chen, Y. Li, D. Zuo, H. Zhang, C. Xiao, J. Chen, J. Diwu, O. Farha, T. Albrecht-Schmitt, Z. Chai, S. Wang, “99TcO4? Remediation by a Cationic Polymeric Network,” Nature Comm. 2018, 9, 3007-3017. DOI: 10.1038/s41467-018-05380-542. S. K. Cary, J. Su, S. S. Galley, T. E. Albrecht-Schmitt, E. R. Batista, M. G. Ferrier, S. A. Kozimor, V. Mocko, B. L. Scott, C. E. Van Alstine, F. D. White, P. Yang, “A Series of Dithiocarbamates for Americium, Curium, and Californium,” Dalton Transactions 2018, 47 (41), 14452-14461, DOI: 10.1039/C8DT02658K41. B. E. Klamm, C. J. Windorff, M. L. Marsh, T. E. Albrecht-Schmitt, “Schiff Base Coordination Complexes with Plutonium(IV) and Cerium(IV),” Chemical Communications 2018, 54, 8634-8626. DOI: 10.1039/C8CC03571G40. A. T. Chemey, C. M. McGuire, T. E. Albrecht-Schmitt, “A Rare Positively-charged Nicotinic Acid Disulfide: 2,2’-dithiodinicotinic Acid Hydrochloride Monohydrate,” Acta Crysta. E 2018, 74, 820-824, DOI: 10.1107/S205698901800691639. Y. Wang, X. Yin, J. Huang, W. Liu, J. Xie, J. Chen, M. A. Silver, D. Sheng, L. Chen, J. Diwu, N. Liu, T. E. Albrecht-Schmitt, Z. Chai, S. Wang, “Emergence of Uranium as a Distinct Metal Center for Building Intrinsic X-ray Scintillators,” Angewandte Chemie., Int. Ed., 2018, DOI: 10.1002/anie.20180286538. Y. Lai, S. E. Bone, M. G. Ferrier, J. Lezama-Pacheco, V. Mocko, A. S. Ditter, S. A. Kozimor, G. T. Seidler, W. L. Nelson, Y.-C. Chiu, K. Huang, W. Potter, D. Graf, T. E. Albrecht-Schmitt, R. E. Baumbach, “Ferromagnetic Quantum Critical Point in CePd2P2 with Pd → Ni Substitution,” Physical Reviews B 2018, 97, 224406. DOI: 10.1103/ PhysRevB.97.22440637. S. S. Galley, A. A. Arico, T.-H. Lee, Y.-X. Yao, X. Deng, J. S. Storbeck, V. Dobrosavljevic, T. E. Albrecht-Schmitt, N. Kaltsoyannis, N. Lanatà, “Uncovering the Origin of Divergence in the CsM(CrO4)2 (M = La, Pr, Nd, Sm, Eu; Am) Family Through Examination of the Chemical Bonding in a Molecular Cluster and by Band Structure Analysis,” J. Amer. Chem. Soc. 2018, 140, 1674-1685. DOI: 10.1021/jacs.7b0947436. Y. Hao, V. Klepov, P. Kegler, G. Modolo, D. Bosbach, T. E. Albrecht-Schmitt, S. Wang, E. Alekseev, “Synthesis and Study of First Zeolitic Uranium Borate,” Crystal Growth & Design 2018, 18, 498-505. DOI: 10.1021/acs.cgd.7b0148735. Y. Hao, V. V. Klepov, P. Kegler, G. Modolo, D. Bosbach, T. E. Albrecht-Schmitt, S. Wang, E. V. Alekseev, “First Zeolite-like Actinide Polyborate,” Crystal Growth & Design 2018, 18, 498–505. DOI: 10.1021/acs.cgd.7b0148734. Y. Wang, H. Lu, X. Dai, X. Bai, Y. Cai, X. Yin, L. Chen, J. Diwu, S. Du, R. Zhou, Z. Chai, T. E. Albrecht-Schmitt, S. Wang, “Facile and Efficient Decontamination of Thorium from Rare Earths based on Selective Selenite Crystallization,” Inorganic Chemistry 2018, 57, 1880-1887. DOI: 10.1021/acs.inorgchem.7b0268133. W. M. Potter, Y. Lai, H. Cao, R. E. Baumbach, S.E. Latturner, “U8Al19Si6, A Uranium Aluminide Silicide with a Stuffed Supercell Grown from Aluminum Flux.” Chem. Mater. 2018, 30, 3806-3812. DOI: 10.1021/acs.chemmater.8b0094832. S. R. Salpage, R. C. Lanzetta, Y. Zhou, J. C. Wang, K. 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Schelter, “Coordination Chemistry of a Strongly-Donating Hydroxylamine with Early Actinides: An Investigation of Redox Properties and Electronic Structure,” Inorg. Chem. 2018, 57, 4387–4394, DOI: 10.1021/acs.inorgchem.7b0323827. K. C. Mullane, T. C. Cheisson, E. Nakamaru-Ogiso, B. C. Manor, P. J. Carroll, E. J. Schelter, “Reduction of Carbonyl Groups by Uranium(III) and Formation of a Stable Amide Radical Anion, Chem. Eur. J. 2018, 24, 826–837. DOI: 10.1002/chem.20170339626. L. Yuan, M. Tian, J. Lan, X. Cao, X. Wang, Z. Chai, J. K. Gibson, W. Shi, “Defect Engineering in Metal–Organic Frameworks: A New Strategy to Develop Applicable Actinide Sorbents,” Chem. Commun. 2018, 54, 370-373 DOI:?10.1039/C7CC07527H.25. X. Wang, Y. Wang, M. A. Silver, D. Gui, Z. Bai, Y. Wang, W. Liu, L. Chen, J. Diwu, Z. Chai, S. Wang, “Superprotonic Conduction Through One-Dimensional Ordered Alkali Metal Ion Chains in a Lanthanide-Organic Framework,” Chem. 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Alekseev, “Divergent Structural Chemistry of Uranyl Borates Obtained from Solid State and Hydrothermal Conditions,” Crystal Growth & Design 2017, 17 (11), 5898-5907 DOI: 10.1021/ acs.cgd.7b00997PATENTS1. K. Hanson, T. E. Albrecht-Schmitt, S. Salpage, 2017, “Photochemical Separations and Compositions,” 2017, WO2019018735A13/30/20 ................
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