SVOC emissions from diesel trucks operating on biodiesel fuels - US EPA
SVOC emissions from diesel trucks operating on biodiesel fuels
Michael D. Hays, William Preston, Ingrid J. George, Pamela Barfield, Bakul Patel, Richard Snow, James Faircloth, Thomas Long, Richard Baldauf, and Joseph McDonald
8/22/2017 Office of Research and Development (ORD)--National Risk Management Research Laboratory (NRMRL)
Motivation
? The 2007 Energy Independence & Security Act (EISA) mandated renewable fuel use in the transportation sector ? EPA sets Renewable Fuel Standards (RFS) annually (flexibility) ? 36 billion gallons of renewable fuels by 2022
Volumes Used to Determine the Proposed 2014 Percentage Standards
Category
Volumea
Range
Cellulosic biofuel
17x106 gal
8-30x106 gallons
Biomass-based diesel (FAMEs)
1.3x109 gal
1.3x109 galb
Advanced biofuel (non-corn EtOH)
2.2x109 gal
2.0-2.5x109 gal
Renewable fuel
15.2x109 gal
15.0-15.5x109 gal
aAll volumes are ethanol-equivalent, except for biomass-based diesel which is actual bEPA is requesting comment on alternative approaches and higher volumes
? As part of these requirements, EPA must: ? Assess the impacts of changes in ethanol volume and other fuel properties on emissions and ambient concentrations of air toxics and criteria pollutants ? Ensure "anti-backsliding" of air quality impacts and propose regulations to mitigate any adverse air quality
2 impacts
otaq/fuels/renewablefuels
Biodiesel study facts
? Roughly, 150 x 109 L of on-highway diesel produced annually in the U.S. of which 5 x 109 is biodiesel ? In many cases, biodiesel use actually reduces criteria pollutant emissions ? Water-soluble OC in PM can increase producing toxicological concerns ? To date, limited emphasis on the gas-phase SVOC emissions and the effect of increasing fuel oxidants ? MOVES model requires emissions information from this engine class ? As of 2016, greater than half of all vehicle miles travelled were for trucks with catalytic control for NOx and PM.
3
MOVES ? Motor Vehicle Emissions Simulator
Diesel emissions control history
active regeneration
passive regeneration
PM 0.10 NOx 4.0 HC 1.3
PM 0.01 NOx 2.5 NMHC 0.50
PM 0.01 NOx 1.4 NMHC 0.14
PM 0.01 NOx 0.20 NMHC 0.14
PM 0.01 NOx 0.20 NMHC 0.14
DOC
DOC
CDPF
SCR
DOC Fuel Injection
CDPF
SCR
Urea Injection Fuel Injection
AMOX Urea Injection
CDPF DOC Fuel Injection
Optional
1998
2004
2007
2010 L/MHDDE
2010 M/HHDDE 4
Experimental ? HD Vehicles (6.7L)
George et al. (2014) ES&T, Vol. 48, Iss. 24, p. 14782
? 2011 Dodge Ram 2500 ? GVWR = 9,600 lb ? DOC/NAC/CDPF ? 35,498 km ? HDV2B
? 2011 Ford F550 ? GVWR = 19,500 lb ? DOC/SCR/CDPF ? 4,333 km ? HDV5
? 2011 Ford F750 ? GVWR = 25,999 lb ? DOC/SCR/CDPF ? 5850 km ? HDV6
Active CDPF regeneration
5
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